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processes on zero-valent iron modified biochar in copper(II) immobilization: from batch solution to pilot-scale

《化学科学与工程前沿（英文）》 2023年 第17卷 第7期   页码 880-892 doi: 10.1007/s11705-022-2282-8

摘要： The zero-valent iron modified biochar materials are widely employed for heavy metals immobilization. However, these materials would be inevitably aged by natural forces after entering into the environment, while there are seldom studies reported the aging effects of zero-valent iron modified biochar. In this work, the hydrogen peroxide and hydrochloric acid solution were applied to simulate aging conditions of zero-valent iron modified biochar. According to the results, the adsorption capacity of copper(II) contaminants on biochar, zero-valent iron modified biochar-1, and zero-valent iron modified biochar-2 after aging was decreased by 15.36%, 22.65% and 23.26%, respectively. The surface interactions were assigned with chemisorption occurred on multi-molecular layers, which were proved by the pseudo-second-order and Langmuir models. After aging, the decreasing of capacity could be mainly attributed to the inhibition of ion-exchange and zero-valent iron oxidation. Moreover, the plant growth and soil leaching experiments also proved the effects of aging treatment, the zero-valent iron modified biochar reduced the inhibition of copper(II) bioavailability and increased the mobility of copper(II) after aging. All these results bridged the gaps between bio-adsorbents customization and their environmental behaviors during practical agro-industrial application.

关键词： zero-valent iron modified biochar     aging processes     copper removal     adsorption     pilot-scale experiments    

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Removal of arsenic by pilot-scale vertical flow constructed wetland

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-021-1435-1

摘要：

• VFCWs are effective for the treatment of arsenic-containing wastewater.

关键词： Constructed wetland     Arsenic     Removal efficiency     Mass balance    

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arsenic capture by a calcium-based sorbent during the combustion of arsenic-contaminated biomass: A pilot-scale

Mei Lei, Ziping Dong, Ying Jiang, Philip Longhurst, Xiaoming Wan, Guangdong Zhou

《环境科学与工程前沿（英文）》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1110-y

摘要：

Pilot-scale combustion is required to treat arsenic-enriched biomass in China.

CaO addition to arsenic-enriched biomass reduces arsenic emission.

CaO captures arsenic via chemical adsorption to form Ca3(AsO4)2.

关键词： Arsenic contamination     Phytoremediation     Emission control     Calcium-based sorbent     Biomass disposal     Pilot-scale combustion    

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Flow characteristic and wastewater treatment performance of a pilot-scale airlift oxidation ditch

Hongtao PANG, Hanchang SHI, Huiming SHI,

《环境科学与工程前沿（英文）》 2009年 第3卷 第4期   页码 470-476 doi: 10.1007/s11783-009-0143-z

摘要： A pilot-scale airlift oxidation ditch using bubble diffuser and baffle as aerator was operated in a wastewater treatment plant (WWTP) to investigate its flow characteristic and wastewater treatment performance. Compared with the conventional oxidation ditch process, effective depth and oxygen utilization efficiency of this new process was improved by underwater aeration. Furthermore, it had a reversed velocity distribution, which decreased from the bottom to the top on vertical section. Velocity measurement showed that a velocity over 0.2m/s at the bottom was sufficient to prevent sludge settlement during long term operation. Application of these concepts would save land area and energy consumption by about 25%―50% and 55%, respectively. In this new system, organic biodegradation and nitrification could be well achieved. Denitrification could occur steadily in the straight part by adjusting the airflow rate. An average TN removal rate of 63% was achieved with dissolved oxygen (DO) concentrations between 0.6mg/L and 1.5mg/L. The main pollutants in the effluent could meet the strictest discharge standard (COD<50mg/L, NH―N<5mg/L, and TN<15mg/L) in China now.

关键词： airlift oxidation ditch     flow characteristic     wastewater treatment    

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Advanced nitrogen removal using pilot-scale SBR with intelligent control system built on three layer

YANG Qing, WANG Shuying, YANG Anming, GUO Jianhua, BO Fengyang

《环境科学与工程前沿（英文）》 2007年 第1卷 第1期   页码 33-38 doi: 10.1007/s11783-007-0006-4

摘要： Since eutrophication has become increasingly severe in China, nitrogen and phosphorous have been the concern of wastewater treatment, especially nitrogen removal. The stabilization of the intelligent control system and nitrogen removal efficiency were investigated in a pilot-scale aerobic-anoxic sequencing batch reactor (SBR) with a treatment capacity of 60 m/d. Characteristic points on the profiles of dissolved oxygen (DO), pH, and oxidation reduction potential (ORP) could exactly reflect the process of nitrification and denitrification. Using the intelligent control system not only could save energy, but also could achieve advanced nitrogen removal. Applying the control strategy water quality of the effluent could stably meet the national first discharge standard during experiment of 10 months. Even at low temperature ( = 13vH), chemical oxygen demand (COD) and total nitrogen (TN) in the effluent were under 50 and 5 mg/L, respectively.

关键词： eutrophication     pilot-scale aerobic-anoxic     stabilization     oxidation reduction     nitrification    

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Feedforward control for nitrogen removal in a pilot-scale anaerobic-anoxic-oxic plant for municipal wastewater

Tonggang SHEN, Hanchang SHI, Huiming SHI, He JING, Huilei XIONG

《环境科学与工程前沿（英文）》 2011年 第5卷 第1期   页码 130-139 doi: 10.1007/s11783-010-0266-2

摘要： To improve the efficiency of nitrogen removal with lower energy consumption, the study of feedforward control was carried out on a pilot-scale anaerobic-anoxic-oxic (AAO) plant for the treatment of municipal wastewater. The effluent qualities of the pilot plant under different control strategies were investigated. The results indicated that the change of external recycle was not a suitable approach to regulate the sludge concentration of plug-flow reactors; adjusting the aeration valve and dissolved oxygen set-point according to ammonia load could overcome the impact of influent fluctuation; and the denitrification potential could be estimated based on the transit time of anoxic zone and the relative content of carbon resource entering the anoxic zone. Simple feedforward control strategies for aeration and internal recycle were subsequently proposed and validated. The nitrogen removal was successfully improved in the pilot plant. The effluent total nitrogen had decreased by 29.9% and was steadily controlled below 15 mg·L . Furthermore, approximately 38% of the energy for aeration had been saved.

关键词： anaerobic-anoxic-oxic (AAO)     feedforward control     municipal wastewater     nitrogen removal    

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Bioreduction of nitrate in groundwater using a pilot-scale hydrogen-based membrane biofilm reactor

Youneng TANG, Michal ZIV-EL, Chen ZHOU, Jung Hun SHIN, Chang Hoon AHN, Bruce E. RITTMANN, Kerry MEYER, Daniel CANDELARIA, David FRIESE, Ryan OVERSTREET, Rick SCOTT,

《环境科学与工程前沿（英文）》 2010年 第4卷 第3期   页码 280-285 doi: 10.1007/s11783-010-0235-9

摘要： A long-term pilot-scale H-based membrane biofilm reactor (MBfR) was tested for removal of nitrate from actual groundwater. A key feature of this second-generation pilot MBfR is that it employed lower cost polyester hollow fibers and still achieved high loading rate. The steady-state maximum nitrate surface loading at which the effluent nitrate and nitrite concentrations were below the Maximum Contaminant Level (MCL) was at least 5.9 g·N·(m·d), which corresponds to a maximum volumetric loading of at least 7.7 kg·N·(m·d) . The steady-state maximum nitrate surface area loading was higher than the highest nitrate surface loading reported in the first-generation MBfRs using composite fibers (2.6 g·N·(m·d)). This work also evaluated the H-utilization efficiency in MBfR. The measured H supply rate was only slightly higher than the stoichiometric H-utilization rate. Thus, H utilization was controlled by diffusion and was close to 100% efficiency, as long as biofilm accumulated on the polyester-fiber surface and the fibers had no leaks.

关键词： denitrification     groundwater treatment     hydrogen     membrane biofilm reactor (MBfR)     polyester fiber    

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Pilot-scale studies of domestic wastewater treatment by typical constructed wetlands and their greenhouse

Chaoxiang LIU, Kaiqin XU, Ryuhei INAMORI, Yuhei INAMORI, Yoshitaka EBIE, Jie LIAO,

《环境科学与工程前沿（英文）》 2009年 第3卷 第4期   页码 477-482 doi: 10.1007/s11783-009-0155-8

摘要： Three typical constructed wetlands (CWs) including Vertical Flow (VF), Free Water Surface (FWS), and Subsurface Flow (SF), and combined VF-SF-FWS constructed wetlands were investigated for the treatment of domestic wastewater with low C/N ratio. The performance of nutrient removal and the characteristics of greenhouse gas emissions, such as CH and NO, from these CWs were compared. The results indicated that the four types of CWs had high removal efficiencies for organic matter and suspended solid (SS). The combined wetland also showed a comparatively good performance for nitrogen and phosphorus removal, and the removal efficiencies for total nitrogen (TN) and total phosphorus (TP) were 81.3% and 84.5%, respectively. The combined CWs had a comparative lower global warming potential. The FWS CW had the highest tendency to emit CH and led to a higher global warming potential among the four types of CWs, which was about 586 mg CO/m·h.

关键词： global warming potential     methane     nitrous oxide     low C/N ratio     nitrogen     phosphorus    

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Dewatering of Scenedesmus Obliquus Cultivation Substrate with Microfiltration: Potential and Challenges for Water Reuse and Effective Harvesting

Marco Malaguti,Lorenzo Craveri,Francesco Ricceri,Vincenzo Riggio,Mariachiara Zanetti,Alberto Tiraferri,

《工程（英文）》 doi: 10.1016/j.eng.2023.07.010

摘要： In the microalgae harvesting process, which includes a step for dewatering the algal suspension, directly reusing extracted water in situ would decrease the freshwater footprint of cultivation systems. Among various algae harvesting techniques, membrane-based filtration has shown numerous advantages. This study evaluated the reuse of permeate streams derived from Scenedesmus obliquus (S. obliquus) biomass filtration under bench-scale and pilot-scale conditions. In particular, this study identified a series of challenges and mechanisms that influence the water reuse potential and the robustness of the membrane harvesting system. In a preliminary phase of this investigation, the health status of the initial biomass was found to have important implications for the harvesting performance and quality of the permeate stream to be reused; healthy biomass ensured better dewatering performance (i.e., higher water fluxes) and higher quality of the permeate water streams. A series of bench-scale filtration experiments with different combinations of cross-flow velocity and pressure values were performed to identify the operative conditions that would minimize energy requirements while maximizing water productivity. The optimal conditions, 2.2 m·s−1 and 1.4 bar (1 bar = 105 Pa), respectively, were then applied to drive pilot-scale microfiltration tests to reuse the collected permeate as a new cultivation medium for S. obliquus growth in a pilot-scale photo-bioreactor. The investigation revealed key differences between the behavior of the membrane systems at the two scales (bench and pilot). It indicated the potential for beneficial reuse of the permeate stream as the pilot-scale experiments ensured high harvesting performance and growth rates of biomass in permeate water that were highly similar to those recorded in the ideal cultivation medium. Finally, different nutrient reintegration protocols were investigated, revealing that both macro- and micronutrient levels are critical for the success of the reuse approach.

关键词： Scenedesmus obliquus     Microfiltration     Permeate reuse     Harvesting     Microalgae     Pilot-scale    

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A pilot scale test of ozonization treatment of ethene wastewater for reuse

ZHONG Li, REN Wei, GUO Wenjing

《化学科学与工程前沿（英文）》 2008年 第2卷 第2期   页码 191-195 doi: 10.1007/s11705-008-0028-x

摘要： A pilot scale test of advanced treatment of ethene wastewater by ozonization was carried out for industrial water reuse. Effects of different operating conditions on COD degradation, such as wastewater flow rate, ozonized gas flow rate, operating voltage of ozonizer and two ozone generation means, using pure oxygen or air, was investigated. The results show that the increase of ozonizer operating voltage, the decrease of wastewater flow rate and the suitable ozonized gas flow rate improve the removal of COD in wastewater and that ozone generated respectively from air and pure oxygen can effectively remove COD of ethene wastewater to meet the industrial water reuse criterion.

关键词： different     industrial     oxygen     generation     criterion    

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Optimizing the configuration of a clearwell by integrating pilot and full-scale tracer testing

LIU Wenjun, DU Zhipeng, JIN Junwei

《环境科学与工程前沿（英文）》 2007年 第1卷 第3期   页码 270-275 doi: 10.1007/s11783-007-0045-x

摘要： In this paper, the main factors impacting the plug flow pattern of a clearwell were investigated by integrating pilot-scale, full-scale clearwell tracer testing and computational fluid dynamics (CFD) simulation. It was found that pilot tracer testing, full-scale tracer testing and CFD simulation all demonstrated that the correlation between the ratio of / and can be approximately expressed by: / = 0.189 4ln()-0.049 4. This study confirmed that the installation of baffles within clearwells is an efficient way to optimize their configuration. In addition, the inlet velocity has a minimal contribution to the ratio of /. However, the ratio of turning channel width to channel width () significantly contributes to the ratio of/. The optimal ratio of is 0.8–1.2 for maintaining better plug flow pattern. The number of turning channels is one of the main factors that impact the ratio of /. When increasing the number of turning channels, a lower ratio of / is obtained.
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On the added value of multi-scale modeling of concrete

《结构与土木工程前沿（英文）》 2022年 第16卷 第1期   页码 1-23 doi: 10.1007/s11709-021-0790-0

摘要： This review of the added value of multi-scale modeling of concrete is based on three representative examples. The first one is concerned with the analysis of experimental data, taken from four high-dynamic tests. The structural nature of the high-dynamic strength increase can be explained by using a multi-scale model. It accounts for the microstructure of the specimens. The second example refers to multi-scale thermoelastic analysis of concrete pavements, subjected to solar heating. A sensitivity analysis with respect to the internal relative humidity (RH) of concrete has underlined the great importance of the RH for an assessment of the risk of microcracking of concrete. The third example deals with multi-scale structural analysis of a real-scale test of a segmental tunnel ring. It has turned out that multi-scale modeling of concrete enables more reliable predictions of crack opening displacements in tunnel segments than macroscopic models taken from codes of practice. Overall, it is concluded that multi-scale models have indeed a significant added value. However, its degree varies with these examples. In any case, it can be assessed by means of a comparison of the results from three sources, namely, multi-scale structural analysis, conventional structural analysis, and experiments.

关键词： experiments     multi-scale analysis     conventional structural analysis     concrete     reinforced concrete    

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process and sulfide precipitation for removal of heavy metals from industrial wastewater: Bench and pilotscale studies focusing on in-depth thallium removal

Huosheng Li, Hongguo Zhang, Jianyou Long, Ping Zhang, Yongheng Chen

《环境科学与工程前沿（英文）》 2019年 第13卷 第4期 doi: 10.1007/s11783-019-1130-7

摘要：

Addition of alkali to pH 10 is effective for precipitation of precipitable metals.

Fenton treatment is effective for substantial removal of Tl, Cd, Cu, Pb, and Zn.

Sulfide precipitation is a final step for removal of trace Tl, Cd, Cu, Pb, and Zn.

Bench and pilot studies demonstrated the effectiveness of this combined technique.

关键词： Thallium     Pilot     Fenton     Sulfide precipitation     Heavy metal     Industrial wastewater    

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Online control of biofilm and reducing carbon dosage in denitrifying biofilter: pilot and full-scale

Xiuhong Liu, Hongchen Wang, Qing Yang, Jianmin Li, Yuankai Zhang, Yongzhen Peng

《环境科学与工程前沿（英文）》 2017年 第11卷 第1期 doi: 10.1007/s11783-017-0895-9

摘要： Online control of DNBF was studied in the pilot-scale and full-scale experiments. DNBF was controlled by the online monitored effluent nitrate and turbidity. The effluent nitrate lower than 3 mg·L and saving 18% of carbon were both achieved. Denitrifying biofilter (DNBF) is widely used for advanced nitrogen removal in the reclaimed wastewater treatment plants (RWWTPs). Manual control of DNBF easily led to unstable process performance and high cost. Consequently, there is a need to automatic control of two decisive operational processes, carbon dosage and backwash, in DNBF. In this study, online control of DNBF was investigated in the pilot-scale DNBF (600 m ·d ), and then applied in the full-scale DNBF (10 × 104 m3·d ). A novel simple online control strategy for carbon dosage with the effluent nitrate as the sole control parameter was designed and tested in the pilot-scale DNBF. Backwash operation was optimized based on the backwash control strategy using turbidity as control parameter. Using the integrated control strategy, in the pilot-scale DNBF, highly efficient nitrate removal with effluent TN level lower than 3 mg·L was achieved and DNBF was not clogged any more. The online control strategy for carbon dosage was successfully applied in a RWWTP. Using the online control strategy, the effluent nitrate concentration was controlled relatively stable and carbon dosage was saved for 18%.

关键词： Reclaimed water treatment     Denitrifying biofilter     Carbon dosage     Backwash control    

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Anoxic phosphorus removal in a pilot scale anaerobic-anoxic oxidation ditch process

Hongxun HOU, Shuying WANG, Yongzhen PENG, Zhiguo YUAN, Fangfang YIN, Wang GAN

《环境科学与工程前沿（英文）》 2009年 第3卷 第1期   页码 106-111 doi: 10.1007/s11783-009-0005-8

摘要： The anaerobic-anoxic oxidation ditch (A /O OD) process is popularly used to eliminate nutrients from domestic wastewater. In order to identify the existence of denitrifying phosphorus removing bacteria (DPB), evaluate the contribution of DPB to biological nutrient removal, and enhance the denitrifying phosphorus removal in the A /O OD process, a pilot-scale A /O OD plant (375 L) was conducted. At the same time batch tests using sequence batch reactors (12 L and 4 L) were operated to reveal the significance of anoxic phosphorus removal. The results indicated that: The average removal efficiency of COD, , , and TN were 88.2%, 92.6%, 87.8%, and 73.1%, respectively, when the steady state of the pilot-scale A /O OD plant was reached during 31-73 d, demonstrating a good denitrifying phosphorus removal performance. Phosphorus uptake took place in the anoxic zone by poly-phosphorus accumulating organisms could be used as electron receptors in denitrifying phosphorus removal, and the phosphorus uptake rate with as the electron receptor was higher than that with when the initial concentration of either or was 40 mg/L.

关键词： wastewater treatment     anaerobic-anoxic (A2/O)     oxidation ditch (OD)     biological phosphorus removal     denitrifying phosphorus removal    

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标题 作者 时间 类型 操作

processes on zero-valent iron modified biochar in copper(II) immobilization: from batch solution to pilot-scale

期刊论文

Removal of arsenic by pilot-scale vertical flow constructed wetland

期刊论文

arsenic capture by a calcium-based sorbent during the combustion of arsenic-contaminated biomass: A pilot-scale

Mei Lei, Ziping Dong, Ying Jiang, Philip Longhurst, Xiaoming Wan, Guangdong Zhou

期刊论文

Flow characteristic and wastewater treatment performance of a pilot-scale airlift oxidation ditch

Hongtao PANG, Hanchang SHI, Huiming SHI,

期刊论文

Advanced nitrogen removal using pilot-scale SBR with intelligent control system built on three layer

YANG Qing, WANG Shuying, YANG Anming, GUO Jianhua, BO Fengyang

期刊论文

Feedforward control for nitrogen removal in a pilot-scale anaerobic-anoxic-oxic plant for municipal wastewater

Tonggang SHEN, Hanchang SHI, Huiming SHI, He JING, Huilei XIONG

期刊论文

Bioreduction of nitrate in groundwater using a pilot-scale hydrogen-based membrane biofilm reactor

Youneng TANG, Michal ZIV-EL, Chen ZHOU, Jung Hun SHIN, Chang Hoon AHN, Bruce E. RITTMANN, Kerry MEYER, Daniel CANDELARIA, David FRIESE, Ryan OVERSTREET, Rick SCOTT,

期刊论文

Pilot-scale studies of domestic wastewater treatment by typical constructed wetlands and their greenhouse

Chaoxiang LIU, Kaiqin XU, Ryuhei INAMORI, Yuhei INAMORI, Yoshitaka EBIE, Jie LIAO,

期刊论文

Dewatering of Scenedesmus Obliquus Cultivation Substrate with Microfiltration: Potential and Challenges for Water Reuse and Effective Harvesting

Marco Malaguti,Lorenzo Craveri,Francesco Ricceri,Vincenzo Riggio,Mariachiara Zanetti,Alberto Tiraferri,

期刊论文

A pilot scale test of ozonization treatment of ethene wastewater for reuse

ZHONG Li, REN Wei, GUO Wenjing

期刊论文

Optimizing the configuration of a clearwell by integrating pilot and full-scale tracer testing

LIU Wenjun, DU Zhipeng, JIN Junwei

期刊论文

On the added value of multi-scale modeling of concrete

期刊论文

process and sulfide precipitation for removal of heavy metals from industrial wastewater: Bench and pilotscale studies focusing on in-depth thallium removal

Huosheng Li, Hongguo Zhang, Jianyou Long, Ping Zhang, Yongheng Chen

期刊论文

Online control of biofilm and reducing carbon dosage in denitrifying biofilter: pilot and full-scale

Xiuhong Liu, Hongchen Wang, Qing Yang, Jianmin Li, Yuankai Zhang, Yongzhen Peng

期刊论文

Anoxic phosphorus removal in a pilot scale anaerobic-anoxic oxidation ditch process

Hongxun HOU, Shuying WANG, Yongzhen PENG, Zhiguo YUAN, Fangfang YIN, Wang GAN

期刊论文